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Although twenty three isotopes of phosphorus are known (all the possible isotopes from 24P up to 46PAnalytical Chemistry Chemistry Question

Radioactive decay

Although twenty three isotopes of phosphorus are known (all the possible isotopes from 24P up to 46P), only 31P, with spin 1/2, is stable and is therefore present at 100% abundance. The half-integer spin and high abundance of 31P make it useful for nuclear magnetic resonance (NMR) spectroscopic studies of bio-molecules, particularly DNA. [1]

Two radioactive isotopes of phosphorus have half-lives that make them useful for scientific experiments. 32P has a half-life of 14.3 days and 33P has a half-life of 25.3 days. Both radioisotopes of phosphorous, 32P and 33P, are beta emitters and they decay as shown in the following nuclear reactions; [2]

^{32}_{15}P → ^{32}_{16}S + beta^-
^{33}_{15}P → ^{33}_{16}S + beta^-

Isotope isotopic masses:
32P: 31.97390727
33P: 32.9717255
32S: 31.97207100
33S: 32.97145876 [3]

23.1.

Calculate the energy of β particles emitted in the decay reactions of 32P and 33P. [2]

Model Answer

For the decay of 32P the mass difference is:
Δm = 31.97390727 - 31.97207100 = 0.00183627 amu
ΔE = Δm c^2 = (1.0 * 10^-3 kg * 0.00183627 amu / (6.0221 * 10^23 amu)) * (2.9979 * 10^8 m/s)^2 = 2.740456 * 10^-13 J
Therefore, for the decay of 32P:
ΔE = 2.740456 * 10^-13 J * (1 eV / 1.602 * 10^-19 J) = 1.7106 * 10^6 eV. [3, 4]

For the decay of 33P, the mass difference is:
Δm = 32.9717255 - 32.97145876 = 0.00026674 amu
ΔE = (1.0 * 10^-3 kg * 0.00026674 amu / (6.0221 * 10^23 amu)) * (2.9979 * 10^8 m/s)^2 = 3.98084 * 10^-14 J
Therefore, for the decay of 33P:
ΔE = 3.98084 * 10^-14 J * (1 eV / 1.602 * 10^-19 J) = 0.248 * 10^6 eV. [4]

23.2.

To shield beta radiation usually lead is used. However, secondary emission of X-rays takes place via a process known as Bremsstrahlung in the case of high energy β-emission. Therefore shielding must be accomplished with low density materials, e.g. Plexiglas, Lucite, plastic, wood, or water. During shielding of β-emission from 32P, X-ray photons of λ = 0.1175 nm are produced. Calculate the energy of X-ray photons in eV. [2, 5]

Model Answer

E = h v = h c / λ
E = (6.6261 * 10^-34 J s * 2.9979 * 10^8 m/s) / (0.1175 * 10^-9 m) = 1.691 * 10^-15 J
Energy of X-ray photons in eV:
E = 1.691 * 10^-15 J * (1 eV / 1.602 * 10^-19 J) = 1.055 * 10^4 eV. [4, 6]

23.3.

Find the mass of 32P which has activity of 0.10 Ci (1 Ci = 3.7·1010 disintegration/s). [5]

Model Answer

A = k N
Activity = 0.10 Ci * (3.7 * 10^10 disintegrations / (s * 1 Ci)) = 3.7 * 10^9 disintegrations / s
Half-life for 32P is 14.3 days = 1.24 * 10^6 s.
k = ln 2 / t_1/2 = ln 2 / (1.24 * 10^6 s) = 5.61 * 10^-7 s^-1
N = A / k = 3.7 * 10^9 s^-1 / (5.61 * 10^-7 s^-1) = 6.6 * 10^15 32P nuclei
n(32P) = 6.6 * 10^15 nuclei / (6.0221 * 10^23 nuclei/mol) = 1.10 * 10^-8 mol
m(32P) = 1.10 * 10^-8 mol * 31.974 g/mol = 3.50 * 10^-7 g. [6, 7]

23.4.

A sample containing both radioisotopes 32P and 33P has an initial activity of 9136.2 Ci. If the activity decreases to 4569.7 Ci after 14.3 days, calculate the 32P/33P ratio initially present in the sample. [3, 5]

Model Answer

Decay constant for 32P = ln 2 / 14.3 day = 4.85 * 10^-2 day^-1
Decay constant for 33P = ln 2 / 25.3 day = 2.74 * 10^-2 day^-1
Let activity of 32P = A32 and activity of 33P = A33
Initially: A32 + A33 = 9136.2 Ci (Equation I)
After 14.3 days, total activity:
Atotal = A32 * e^(-k32 * t) + A33 * e^(-k33 * t)
Atotal = A32 * e^(-0.0485 * 14.3) + A33 * e^(-0.0274 * 14.3)
Atotal = 0.50 * A32 + 0.675 * A33 = 4569.7 Ci (Equation II)

Solving Equation I and II gives:
A33 = 9.12 Ci and A32 = 9127.3 Ci

Thus, the initial 32P / 33P nuclei ratio is:
N32 / N33 = (A32 * k33) / (A33 * k32) = (9127.3 * 2.74 * 10^-2) / (9.12 * 4.85 * 10^-2) = 5.63 * 10^2. [7, 8]

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